Alloyed (ZnS)x(CuInS2)(1-x) semiconductor nanorods: synthesis, bandgap tuning and photocatalytic properties.
Identifieur interne : 001002 ( Main/Exploration ); précédent : 001001; suivant : 001003Alloyed (ZnS)x(CuInS2)(1-x) semiconductor nanorods: synthesis, bandgap tuning and photocatalytic properties.
Auteurs : RBID : pubmed:22865784English descriptors
- KwdEn :
- MESH :
- chemical , chemical synthesis : Colloids.
- chemical , chemistry : Colloids, Copper, Indium, Sulfides, Zinc Compounds.
- chemistry : Nanotubes.
- Catalysis, Photochemical Processes, Semiconductors.
Abstract
Rod-like nanocrystals of the semiconductor alloy (ZnS)(x)(CuInS(2))(1-x) (ZCIS) have been colloidally prepared by using a one-pot non-injection-based synthetic strategy. The ZCIS nanorods crystallize in the hexagonal wurtzite structure and display preferential growth in the direction of the c axis. The bandgap of these quarternary alloyed nanorods can be conveniently tuned by varying the ratio of ZnS to CuInS(2). A non-linear relationship between the bandgap and the alloy composition is observed. The ZCIS nanorods are found to exhibit promising photocatalytic behaviour in visible-light-driven degradation of Rhodamine B.
DOI: 10.1002/chem.201201626
PubMed: 22865784
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The ZCIS nanorods crystallize in the hexagonal wurtzite structure and display preferential growth in the direction of the c axis. The bandgap of these quarternary alloyed nanorods can be conveniently tuned by varying the ratio of ZnS to CuInS(2). A non-linear relationship between the bandgap and the alloy composition is observed. The ZCIS nanorods are found to exhibit promising photocatalytic behaviour in visible-light-driven degradation of Rhodamine B.</div></front></TEI><pubmed><MedlineCitation Owner="NLM" Status="MEDLINE"><PMID Version="1">22865784</PMID><DateCreated><Year>2012</Year><Month>08</Month><Day>28</Day></DateCreated><DateCompleted><Year>2012</Year><Month>12</Month><Day>28</Day></DateCompleted><DateRevised><Year>2013</Year><Month>11</Month><Day>21</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1521-3765</ISSN><JournalIssue CitedMedium="Internet"><Volume>18</Volume><Issue>36</Issue><PubDate><Year>2012</Year><Month>Sep</Month><Day>3</Day></PubDate></JournalIssue><Title>Chemistry (Weinheim an der Bergstrasse, Germany)</Title><ISOAbbreviation>Chemistry</ISOAbbreviation></Journal><ArticleTitle>Alloyed (ZnS)x(CuInS2)(1-x) semiconductor nanorods: synthesis, bandgap tuning and photocatalytic properties.</ArticleTitle><Pagination><MedlinePgn>11258-63</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1002/chem.201201626</ELocationID><Abstract><AbstractText>Rod-like nanocrystals of the semiconductor alloy (ZnS)(x)(CuInS(2))(1-x) (ZCIS) have been colloidally prepared by using a one-pot non-injection-based synthetic strategy. The ZCIS nanorods crystallize in the hexagonal wurtzite structure and display preferential growth in the direction of the c axis. The bandgap of these quarternary alloyed nanorods can be conveniently tuned by varying the ratio of ZnS to CuInS(2). A non-linear relationship between the bandgap and the alloy composition is observed. The ZCIS nanorods are found to exhibit promising photocatalytic behaviour in visible-light-driven degradation of Rhodamine B.</AbstractText><CopyrightInformation>Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Ye</LastName><ForeName>Chen</ForeName><Initials>C</Initials><Affiliation>Institute of Materials Research and Engineering, Agency for Science, Technology and Research (A*STAR), 3 Research Link, 117602 Singapore.</Affiliation></Author><Author ValidYN="Y"><LastName>Regulacio</LastName><ForeName>Michelle D</ForeName><Initials>MD</Initials></Author><Author ValidYN="Y"><LastName>Lim</LastName><ForeName>Suo Hon</ForeName><Initials>SH</Initials></Author><Author ValidYN="Y"><LastName>Xu</LastName><ForeName>Qing-Hua</ForeName><Initials>QH</Initials></Author><Author ValidYN="Y"><LastName>Han</LastName><ForeName>Ming-Yong</ForeName><Initials>MY</Initials></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType>Journal Article</PublicationType><PublicationType>Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2012</Year><Month>08</Month><Day>02</Day></ArticleDate></Article><MedlineJournalInfo><Country>Germany</Country><MedlineTA>Chemistry</MedlineTA><NlmUniqueID>9513783</NlmUniqueID><ISSNLinking>0947-6539</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance>Colloids</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance>Sulfides</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance>Zinc Compounds</NameOfSubstance></Chemical><Chemical><RegistryNumber>045A6V3VFX</RegistryNumber><NameOfSubstance>Indium</NameOfSubstance></Chemical><Chemical><RegistryNumber>789U1901C5</RegistryNumber><NameOfSubstance>Copper</NameOfSubstance></Chemical><Chemical><RegistryNumber>KPS085631O</RegistryNumber><NameOfSubstance>zinc sulfide</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName MajorTopicYN="N">Catalysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Colloids</DescriptorName><QualifierName MajorTopicYN="N">chemical synthesis</QualifierName><QualifierName MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Copper</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Indium</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Nanotubes</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Photochemical Processes</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Semiconductors</DescriptorName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Sulfides</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName MajorTopicYN="N">Zinc Compounds</DescriptorName><QualifierName MajorTopicYN="Y">chemistry</QualifierName></MeshHeading></MeshHeadingList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2012</Year><Month>5</Month><Day>9</Day></PubMedPubDate><PubMedPubDate PubStatus="aheadofprint"><Year>2012</Year><Month>8</Month><Day>2</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2012</Year><Month>8</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2012</Year><Month>8</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2012</Year><Month>12</Month><Day>29</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="doi">10.1002/chem.201201626</ArticleId><ArticleId IdType="pubmed">22865784</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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